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Signature of electronic correlation in multi-electron emission from C60

Kidun, O., Fominykh, N., Berakdar, J.

Chemical Physics Letters 410, pp 293-297 (2005)

Contrasting single to double-particle transition probabilities induced by a one-particle perturbation yields information on the strength of (two-particle) correlation in a system. Here, we calculate single and double ionization probabilities for a C60 molecule upon the absorption of a single photon. We employ the Hartree-Fock and the frozen-core approximations for single-particle states and the random-phase approximation for the screened Coulomb interaction. Energy and angular dependencies of total and differential cross-sections are analyzed and the signature of the geometry of the fullerene and its charge-density response are pointed out.

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